It is also desirable to develop Ge anodes with higher energy and power densities via facile low-cost methods. Efforts should be taken on promoting the practical application of germanium-based anode materials for lithium ion batteries with high power densities.
In addition to the high theoretical capacity, germanium-based materials have many other obvious advantages. 1) High lithium-ion diffusivity. Ge is 400 times faster in lithium ion diffusion than Si (at room temperature, 1.41 × 10−14 cm 2 s −1 for Si and 6.51 × 10 −12 cm 2 s −1 for Ge ; at 150 °C, 3.1 × 10 −9 cm 2 s −1 for Ge) .
In addition, the total citation in 2019 is up to 4892. Fig. 1. Evolution in the number of papers related to germanium-based anode materials for Li-ion batteries, (a) the total publications per year and (b) sum of times cited per year. (Data source: Web of Science, 23-April-2020).
1. Introduction Lithium ion batteries (LIBs) with advanced properties, such as high energy and power densities, low cost, and long cycling span, have received tremendous consideration in the past decade [1, 2]. Nowadays, LIBs have been successfully used in portable electronic devices, power tools and electric vehicles.
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